Hi Johnny!
So I think this is rather interesting because it reminds of 17,18, and 19th century illustrations of Mephistopheles from Goethe’s (or Christopher Marlowe’s or just the fairy tale of) Faust, about the doctor who sold his souls to the devil for wishes, riches, and the woman of his dreams. I would definitely take a look at the famous Mephisto sculpture by 19th century Russian sculptor Mark Antokolsky (link below)
https://en.wikipedia.org/wiki/Mark_Antokolsky#/media/File:Mephisto_by_Mark_Antokolski,_marble_(GTG,_after_1883)_by_shakko_09.jpg
What I recommend is that you focus on the forms of the head, the skull, and of course, major plane breaks. The thing is, that even if you exaggerate the character and features, they still need to correspond to a structured head (and that’s even if it’s more graphic and flat in execution.) So here, for instance, I would make sure the nose is attaching like a pyramidal form to the face, the jaw by the ear is pushed further back from the face, and the ear (even if kept that big) moved down.
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